Spatially heterogeneous dynamics and dynamic facilitation in a model of viscous silica.

نویسندگان

  • Michael Vogel
  • Sharon C Glotzer
چکیده

We perform molecular dynamics simulations to study the structural relaxation dynamics of a model of viscous silica, the prototype of a strong glass former. We find that the melt dynamics are spatially heterogeneous regardless of whether the bulk relaxation is non-Arrhenius or Arrhenius, and cannot be understood as a statistical bondbreaking process. Further, we show that stringlike motion is suppressed by the covalent bondings, yet high particle mobility propagates continuously, supporting the concept of dynamic facilitation emphasized in recent theoretical work.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Temperature dependence of spatially heterogeneous dynamics in a model of viscous silica.

Molecular dynamics simulations are performed to study spatially heterogeneous dynamics in a model of viscous silica above and below the critical temperature of the mode coupling theory, T(MCT) . Specifically, we follow the evolution of the dynamic heterogeneity as the temperature dependence of the transport coefficients shows a crossover from non-Arrhenius to Arrhenius behavior when the melt is...

متن کامل

Effects of Brace-viscous Damper System on the Dynamic Response of Steel Frames

In this study, the effects of three different viscous damper configurations, chevron, diagonal and toggle, as well as brace stiffness on the performance of brace-viscous damper system in various steel frams under different earthquake records were investigated. A finite element software, ANSYS, is exploited to develop the numerical models. To verify the numerical simulations, their results were ...

متن کامل

Examination of dynamic facilitation in molecular dynamics simulations of glass-forming liquids.

Using data from molecular dynamics computer simulations of the one-component Dzugutov liquid and of BKS silica in metastable equilibrium supercooled states, we examine ideas introduced by Garrahan and Chandler (GC) in their dynamic facilitation (DF) model of the glass transition. Utilizing a recently introduced measure of DF, we find that DF is important for particle motion in both the supercoo...

متن کامل

The effect of Proprioceptive Neuromuscular Facilitation exercises on dynamic visual acuity and Sport performance of young basketball players

Aims: Deep sense plays a significant role in sensory control feedback, joint stability, coordination and balance. Despite the important role of vision and Proprioceptive Neuromuscular Facilitation on functional skills in athletes, a few studies have been conducted in this regard. This study aimed at investigating the effects of Proprioceptive Neuromuscular Facilitation exercises on dynamic visu...

متن کامل

Nonlinear Dynamic Buckling of Viscous-Fluid-Conveying PNC Cylindrical Shells with Core Resting on Visco-Pasternak Medium

The use of intelligent nanocomposites in sensing and actuation applications has become quite common over the past decade. In this article, electro-thermo-mechanical nonlinear dynamic buckling of an orthotropic piezoelectric nanocomposite (PNC) cylindrical shell conveying viscous fluid is investigated. The composite cylindrical shell is made from Polyvinylidene Fluoride (PVDF) and reinforced by ...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Physical review letters

دوره 92 25 Pt 1  شماره 

صفحات  -

تاریخ انتشار 2004